To remove the phone-synced files from the laptop without deleting the originals on the phone, do this in order:
- Open Settings on the PC.
- Go to Bluetooth & devices > Mobile devices > Manage devices.
- Turn off Show mobile device in File Explorer.
- Open File Explorer and go to:
C:\Users\<your username>\CrossDevice - Delete the files or folders there that were copied from the phone.
That removes the local copies on the PC and does not affect the files on the phone.
If the phone is still linked and there are ongoing sync issues, reset the connection:
- On the PC, go to Start > Settings > Bluetooth & devices.
- Select Phone Link from the list.
- Toggle Phone Link off and back on.
- Reopen Phone Link.
If that is not enough, fully reset the link:
- On the Android device, go to Settings > Apps > Link to Windows.
- Tap Force Stop.
- On the PC, open Start > Settings > Phone > Unlink this PC.
- Then go to Settings > Apps > Apps & features > Phone Link > Advanced options > Reset.
If the goal is only to stop future syncing, Phone Link also lets features be turned off individually in Phone Link > Settings > Features.
References: