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Thank you for reaching out to the Q&A Forum.
To better understand your situation, could you please share some information:
The Bounce Message: When the email bounces, you should receive a "Non-Delivery Report" (NDR). Could you please share this Error Code or the Diagnostic information for administrators' section here? Usually looks like 550 5.7.1 or mentions specific text like "Unauthenticated email is not accepted". (Note: Please remove any personal email addresses from the text before posting here or you can share a full screenshot via Private Message)
Account Type: Are you sending this from a personal account (ending in @outlook.com, @hotmail.com, @live.com) or a business/custom domain account (ending with @yourbusiness.com hosted by Microsoft 365)?
Group Size: Approximately how many Gmail recipients are in this group?
In the meantime, you can try sending the email to the Gmail recipients in smaller batches (5-10 people at a time) rather than all at once. And if your email signature or body contains links to websites, try sending a plain text test email without links to see if it goes through. Sometimes a specific URL is flagged.
I look forwarding to your response.
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